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Feng, Fu; Wang, Tao; Qiao, Jie; Min, Changjun; Yuan, Xiaocong; Somekh, Michael
Plasmonic and graphene-functionalized high-performance broadband quasi-two-dimensional perovskite hybrid photodetectors Journal Article
In: ACS Appl. Mater. Interfaces, vol. 13, no. 51, pp. 61496–61505, 2021.
Abstract | Tags: film, graphene, light trapping, photodetector, plasmonic, quasi-2D perovskite
@article{Feng2021-bt,
title = {Plasmonic and graphene-functionalized high-performance broadband
quasi-two-dimensional perovskite hybrid photodetectors},
author = {Fu Feng and Tao Wang and Jie Qiao and Changjun Min and Xiaocong Yuan and Michael Somekh},
year = {2021},
date = {2021-12-01},
journal = {ACS Appl. Mater. Interfaces},
volume = {13},
number = {51},
pages = {61496\textendash61505},
publisher = {American Chemical Society (ACS)},
abstract = {Quasi-two-dimensional (2D) layered organic-inorganic hybrid
perovskites have attracted extensive attention, owing to their
excellent optoelectronic tunability and moisture stability
compared with three-dimensional perovskite counterparts and show
great potential for application in photodetectors (PDs).
However, owing to the unavoidable grain boundary defects of
perovskite polycrystalline films, the photocurrent is limited by
poor light absorption and charge mobility. Therefore, the
preparation of quasi-2D perovskite films with strong light
trapping and high charge mobility has been challenging. In this
study, novel broadband quasi-2D perovskite (BA)2(FA)n-1PbnI3n+1
hybrid-structure PDs with good stability were fabricated by
combining both monolayer graphene and Au square nanoarrays. The
hybrid system using both graphene and Au square nanoarrays
effectively improved the carrier mobility and light absorption
and simultaneously maximized light trapping and light-induced
carrier extraction, which resulted in PDs with greatly enhanced
photocurrent in the visible and near-infrared range. The
graphene-Au array-perovskite-based PDs had a low dark current of
10-10 A, large on/off ratio of 104, high responsivity of 18.71 A
W-1, and detectivity of 2.21 $times$ 1013 Jones. The
responsivity and detectivity were two orders of magnitude higher
than those of PDs based only on perovskites. This work
demonstrates a promising and feasible device based on the
coupling of a gold array, layered graphene, and quasi-2D
perovskites, which shows great potential for the development of
high-performance broadband perovskite PDs.},
keywords = {film, graphene, light trapping, photodetector, plasmonic, quasi-2D perovskite},
pubstate = {published},
tppubtype = {article}
}
Qiao, Jie; Feng, Fu; Wang, Ziming; Shen, Mengyan; Zhang, Guoping; Yuan, Xiaocong; Somekh, Michael G
Highly in-plane anisotropic two-dimensional ternary Ta2NiSe5 for polarization-sensitive photodetectors Journal Article
In: ACS Appl. Mater. Interfaces, vol. 13, no. 15, pp. 17948–17956, 2021.
Abstract | Tags: field-effective transistors, in-plane anisotropy, photodetector, polarization-sensitive photodetector, Ta2NiSe5
@article{Qiao2021-cu,
title = {Highly in-plane anisotropic two-dimensional ternary Ta2NiSe5
for polarization-sensitive photodetectors},
author = {Jie Qiao and Fu Feng and Ziming Wang and Mengyan Shen and Guoping Zhang and Xiaocong Yuan and Michael G Somekh},
year = {2021},
date = {2021-04-01},
journal = {ACS Appl. Mater. Interfaces},
volume = {13},
number = {15},
pages = {17948\textendash17956},
publisher = {American Chemical Society (ACS)},
abstract = {Intriguing anisotropic electrical and optoelectrical properties
in two-dimensional (2D) materials are currently gaining
increasing interest both for fundamental research and emerging
optoelectronic devices. Identifying promising new 2D materials
with low-symmetry structures will be rewarding in the
development of polarization-integrated nanodevices. In this
work, the anisotropic electron transport and optoelectrical
properties of multilayer 2D ternary Ta2NiSe5 were systematically
researched. The polarization-sensitive Ta2NiSe5 photodetector
shows a linearly anisotropy ratio of $approx$3.24 with 1064 nm
illumination. The multilayer Ta2NiSe5-based field-effective
transistors exhibit an excellent field-effective mobility of
161.25 cm2·V-1·s-1 along the a axis (armchair direction) as well
as a great current saturation characteristic at room
temperature. These results will promote a better understanding
of the optoelectrical properties and applications in new
categories of the in-plane anisotropic 2D materials.},
keywords = {field-effective transistors, in-plane anisotropy, photodetector, polarization-sensitive photodetector, Ta2NiSe5},
pubstate = {published},
tppubtype = {article}
}
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